Selective C-H Bond Functionalization of Pyrrolo[1,2-a]quinoxaline
Pyrrolo[1,2-a]quinoxalines as important heterocyclic compounds have potential application in pharmaceuticals and synthesis due to their wide range of biological activities and pharmacological effects. This research project focuses on the modification of pyrrolo[1,2-a]quinoxaline as core structure by direct C-H bond functionalization. We expect to obtain a series of efficient approaches for introducing halogen, difluoroacetate, aryl, and arylthio groups on the pyrrolo [1,2-a]quinoxaline, and to reveal the reaction mechanism of C-X bond formation for the direct C-H bond functionalization of pyrrolo[1,2-a]quinoxaline.
Sample Chapter(s)
Preface (89 KB)
Components of the Book:
  • Preface
  • Brief Introduction of the Author
  • Content
  • Chapter 1 Construction of the pyrrolo[1,2-a]quinoxalines skeleton
    • 1. Preparation of pyrrolo[1,2-a]quinoxaline from2-(1H-pyrrol-1-yl)arylamine
    • 2. Preparation of pyrrolo[1,2-a]quinoxaline from1-(2-nitroaryl)-1H-pyrrole
    • 3. Preparation of pyrrolo[1,2-a]quinoxaline from1-(2-isocyanoaryl)-1H-pyrrole
    • 4. Preparation of pyrrolo[1,2-a]quinoxaline form1-(2-Haloaryl)-1H-pyrrole
  • Chapter 2 Selective Halogenation of Pyrrolo[1,2-a]quinoxalines
    • 5. Regioselective Bromination of Pyrrolo[1,2-a]quinoxalines
    • 6. Highly Selective C3-H Iodination of Pyrrolo[1,2-a]quinoxaline
    • 7. Solvent mediated selective C-H bond iodination of pyrrolo[1,2-a]quinoxaline
  • Chapter 3 Metal-Catalyzed C-H activation of Pyrrolo[1,2-a]quinoxalines
    • 8. Cu-Catalyzed Direct C1-H Difluoromethylation of Pyrrolo[1,2-a]quinoxalines
    • 9. Cu-catalyzed direct C1-H trifluoromethylation of pyrrolo[1,2-a]quinoxalines
    • 10. Copper-Promoted C1-H Amination of Pyrrolo[1,2-a]quinoxaline with N-Fluorobenzenesulfonimide
    • 11. Pd-Catalyzed Direct C-H Arylation of Pyrrolo[1,2-a]quinoxalines
    • 12. Ag-catalysed regioselective C1-amidation of pyrrolo[1,2-a]quinoxaline with azodicarboxylates
  • Chapter 4 Metal-free Promoted C-H activation of Pyrrolo[1,2-a]quinoxalines
    • 13. NCS-Promoted Thiocyanation and Selenocyanation of Pyrrolo[1,2-a]quinoxalines
    • 14. I2-Promoted Direct C-H Arylselenylation of Pyrrolo[1,2-a]quinoxalines
    • 15. Metal-free sulfenylation of pyrrolo[1,2-a]quinoxaline with diaryl disulfide facilitated by TBATB
    • 16. KI/TBHP-Promoted [3+2] Cycloaddition of Pyrrolo[1,2-a]quinoxaline and N-Arylsulfonylhydrazones
  • Chapter 5 Direct C-H activation of other N-heterocycles
    • 17. Halogenations of 3-aryl-1H-pyrazol-5-amines
    • 18. TBAI-mediated sulfenylation of polysubstituted 1H-pyrazol-5-amine and arylsulfonyl hydrazide
    • 19. Iodophor-Catalyzed Sulfenylation of Indoles with Sulfonyl Hydrazides for the Synthesis of 3-Sulfenylindoles
    • 20. Iodophor/H2O2 mediated 2-Sulfonylation of Indoles and N-Methylpyrrole in Aqueous Phase
    • 21. Iodophor-catalysed bi-sulfenylation of aminonaphthalenes with arylsulfonyl hydrazines
Readership: Students, academics, teachers and other people attending or interested in Selective C-H Bond Functionalization.
1
Preface
Ping Liu, Yan Liu, He Jing
PDF (89 KB)
3
Brief Introduction of the Author
Ping Liu, Yan Liu, He Jing
PDF (335 KB)
7
Content
Ping Liu, Yan Liu, He Jing
PDF (115 KB)
1
Chapter 1 Construction of the pyrrolo[1,2-a]quinoxalines skeleton
Ping Liu, Yan Liu, He Jing
PDF (344 KB)
9
Chapter 2 Selective Halogenation of Pyrrolo[1,2-a]quinoxalines
Ping Liu, Yan Liu, He Jing
PDF (1326 KB)
55
Chapter 3 Metal-Catalyzed C-H activation of Pyrrolo[1,2-a]quinoxalines
Ping Liu, Yan Liu, He Jing
PDF (1946 KB)
131
Chapter 4 Metal-free Promoted C-H activation of Pyrrolo[1,2-a]quinoxalines
Ping Liu, Yan Liu, He Jing
PDF (1851 KB)
199
Chapter 5 Direct C-H activation of other N-heterocycles
Ping Liu, Yan Liu, He Jing
PDF (1434 KB)
Ping Liu
Ping Liu, Ph.D., Professor, received his Ph.D. degree in Applied Chemistry from Dalian University of Technology in 2010, and joined the School of Chemistry and Chemical Engineering of Shihezi University in the same year. He is a backbone teacher of Corps of Excellence, a university 3152 subject leader, and a backbone member of the Huang Dainian-style teacher team in national universities and colleges.

Yan Liu
Ph.D., professor, received her Ph.D. degree in chemical engineering and technology from Dalian University of Technology in 2010, joined the School of Chemistry and Chemical Engineering of Shihezi University in the same year, and is a 3152 young backbone teacher of Shihezi University, presided over 2 university-level projects, participated in 3 National Natural Science Foundation of China projects.

He Jing
Doctor of Engineering, Senior Laboratory Technician, received her PhD degree in Chemical Engineering and Technology from Shihezi University in June 2022, and joined the School of Chemistry and Chemical Engineering of Shihezi University in the same year, presided over the project of Graduate Student Innovation and Scientific Research Programme of the Autonomous Region.

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