Open Journal of Air Pollution, 2013, 2, 47-55 http://dx.doi.org/10.4236/ojap.2013.23007 Published Online September 2013 (http://www.scirp.org/journal/ojap) A Review of Air Pollution and Control in Hebei Province, China Litao Wang, Jing Yang, Pu Zhang, Xiujuan Zhao, Zhe Wei, Fenfen Zhang, Jie Su, Chenchen Meng Department of Environmental Engineering, Hebei University of Engineering, Handan, China Email: wanglitao@hebeu.edu.cn Received June 19, 2013; revised July 25, 2013; accepted August 1, 2013 Copyright © 2013 Litao Wang et al. This is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. ABSTRACT Hebei is one of the most air polluted provinces in China. According to the Ministry of Environmental Protection (MEP) for the severe fog-haze month of Jan. 2013, seven of the top ten most polluted cities in China are located in Hebei Province. In this study, the air pollution history and status of the Hebei Province are reviewed and discussed, using the governmental published Air Pollution Index (API), the academic observations by various scientific research groups and the long-term statistics of visibility and haze frequencies. It is found that within the Hebei Province, the air pollution in the southern cities is much more severe than the northern cities. Particulate matter (PM) is undoubtedly the major air pollutant, sulfur dioxide (SO2) and nitrogen oxides (NOX) pollutions are also unnegligible. Ozone (O3) pollution in lar- ger cities, such as Shijiazhuang, is significant. Air pollution control history from 1998 is discussed as well. Although Hebei Province has made a great effort on air quality, the pollutant emissions, such as SO2 and fly ash, showed a nota- ble increase in 2001 to 2006. However, after 2006 the emissions started to decrease due to the strict implementation of the national 11th Five Year Plan (FYP). In addition, regional jointly air pollution control and prevention strategies are expected in the future to substantially change the severe air pollution status in Hebei Province. Keywords: Air Quality; Hebei; API; PM2.5 1. Introduction In Jan. 2013, continuous, severe haze pollution hap- pened in east and central China, attracting the most pub- lic attention. In Beijing, only five days were not fog and haze days during Jan. 2013. It is reported that the daily fine particulate matter (PM2.5) concentrations in Beijing and Shijiazhuang has been over 500 μg·m−3, which is 6.7 times of the new China National Ambient Air Quality Standard (CNAAQS) [1]. In the statistics of the Ministry of Environmental Protection of China (MEP), during this month, the ten most polluted cities are Xingtai, Shijiaz- huang, Baoding, Handan, Langfang, Hengshui, Jinan, Tangshan, Beijing and Zhengzhou city, out of the re- ported 74 key cities all over China (http://hebei.sina. com.cn/news/yz/2013-02-06/075733562.html). It should be noted that in these ten top polluted cities, seven cities are within Hebei Province and five of them are located in the southern area of Hebei (see Figure 1). The air pollu- tion in Hebei Province has aroused wide public concern. Hebei Province, located in the north-east of China, is east to the Taihang Mountains and north to the Yellow River (see Figure 1). It encloses two municipal cities, Beijing and Tianjin. The neighboring provinces (in clock- wise direction) are Shandong Province, Henan Province, Shanxi Province, Inner Mongolia Autonomous Region and Liaoning Province. It has the area of 187,700 sq·km and population of 71.85 million (http://www.stats.gov.cn/ tjgb/rkpcgb/dfrkpcgb/t20120228_402804324.htm). Most of the northwest area of Hebei is mountainous or hilly, while the central and south areas belong to North China Plain. Hebei has a monsoon climate of medium latitudes, which has dry and windy springs, hot and rainy summers and dry-cold winters. In 2011, Hebei’s Gross Domestic Product (GDP) is 2.45 trillion RMB, accounting for 5.18% of national GDP and ranking 6th in China [2]. The major industries in Hebei are iron, steel, coke and cement. In 2011, 45.5% of the steel in the world was produced in China, out of which 24.0% was produced in Hebei [2]. China’s coke production accounted for more than 60% of the world, of which 14.5% was produced in Hebei [3]. Hebei’s cement production was 6.9% of the national total amount [2]. The air pollution burden of the southern Hebei area is particularly heavy because of its special location. It is sur- C opyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. 48 B Be ei ij ji in ng g S Sh hi ij ji ia az zh hu ua an ng g T Ti ia an nj ji in n X Xi in ng gt ta ai i H Ha an nd da an n H He en ng gs sh hu ui i C Ca an ng gz zh ho ou u B Ba ao od di in ng g Zhangjiakou Chengde Qinhuangdao T Ta an ng gs sh ha an n L La an ng gf fa an ng g (a) (b) Figure 1. Location of Hebei Province and the cities: (a) locations of Hebei Province in China; (b) eleven cities in Hebei Province. rounded by the other three populated and industrialized provinces, Shandong, Henan and Shanxi. The steel, coke and cement productions of the four neighbored provinces are as large as 40.8%, 50.1% and 22.6% of the national total amount. That is to say, 18.6% of steel production in the world, 30.0% of the coke and 13.6% of the cement were yielded in this area. The large industrial productions induce huge quantities of pollutants emission. In the widely-used Asian INTEX- B emission inventory [4], the PM2.5 emissions from the four provinces accounted for 28% of the national total emission in 2006. The percentages for SO2, NOX, CO, VOC, BC and OC were 28%, 25%, 28%, 24%, 30% and 24%. It gives us a clue why Hebei Province, especially the southern area, has the most severe air pollution all over China. Hebei is somewhat overshadowed by its two neighbors, Beijing and Tianjin. Like other aspects, its air pollution problems haven’t been paid enough attention for a long time. Very few studies have focused on the air pollution status in Hebei area, analyzed the present control strate- gies and given relative suggestions. In the 12th FYP of Air Pollution Control in the Key Regions by MEP at the end of 2012 (http://www.mep.gov.cn/gkml/hbb/bwj/2012 12/t20121205_243271.htm), Beijing, Tianjin and Hebei area is one the three key air pollution control regions and will be pursued regional jointly air pollution prevention and control. Better strategies and more effective actions should be expected in Hebei area. In this paper, we summarize the air quality history and status according to both the governmental reports and the relative academic studies, and also review the air pollution control meas- urements pursued within Hebei area and give suggestions on future pollution control. 2. Air Pollution History and Status 2.1. API and AQI The API is a non dimensional number calculated accord- ing to the urban daily average concentrations of three pollutants: SO2, nitrogen dioxide (NO2) and coarse par- ticulate matter (PM10). Besides of the simplicity, it pro- vided the only publicly accessible urban air quality data before the real time concentrations of the three pollutants of the national sites were started to be published online in 2011. The API record of the key environmental protect- tion cities from 2000 is on the website of the Ministry of Environmental Protection (http://datacenter.mep.gov.cn/). The detailed introduction of API system can be found on in [5]. Before 2003, only Shijiazhuang, the capital city of Hebei was listed in the China’s key environmental pro- tection cities and had the API record on the website of MEP from 2000. In Feb. 2011, three other Hebei cities, Tangshan, Baoding and Handan started to publish their APIs. Figure 2 provides the distribution of the APIs in Shijiazhuang from 2001 to 2012. It can be seen that in general, air quality in Shijiazhuang city was visibly im- proved in 2001 to 2009. The number of the days with the APIs less than or equal to 50 (which is also “no key pol- lutant” day, see [5]) and between 50 - 100 was notably increased from 0 and 93 in 2001, to 43 and 274 in 2012, respectively. And the days having the APIs in 100 - 150 and 150 - 200 decreased, respectively, from 168 and 79 Copyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. 49 in 2001, to 44 and 2 in 2009. The severely polluted days, in which the API was higher than 300, decline from 12 to 0 in 2001 to 2009. After 2009, the pollution level kept relatively stable. The frequencies of the APIs within 150 - 200 even in- creased from 2 days in 2009 to 10 days in 2012 (note that the API less than 100 means the city’s air quality reach the CNAAQS [6]. The annual average APIs were 77.5, 74.6, 75.5, and 74.1 in 2009, 2010, 2011 and 2012, re- spectively. This number is 138.3 in 2001, 91.7 in 2005, and 83.5 in 2008. Figure 3 shows the time series of API in Shijiazhuang city in the past five years. It is shown that the daily varia- tions of APIs were consistent for the five years, that the best air quality appeared in Sep., Aug. and Jul., with the three-month-average APIs of 55.5 (2012) to 66.9 (2008). Then followed Jun., May and Feb. Winter was the worst season that the monthly average APIs were within 69.6 (2010) to 114.0 (2012) for Jan., 78.8 (2011) to 87.8 (2008) for Nov., and 89.1 (2009) to 111.1 (2010) for Dec. In Mar. and Apr. 2008, the APIs indicated two pollution episodes induced by sand storms. Despite the two epi- sodes, the average APIs were 55.9 (2011) to 76.0 (2010) for Mar., and 72.2 (2011) to 89.3 (2009) for Apr. Other information indicated by Figure 3 is that the air quality in Shijiazhuang didn’t show noticeable improvement or deterioration during the recent five years, which is con- sistent with the above discussions. Since February 2011, three other cities, Tangshan, Baoding and Handan started to release their APIs on the website of MEP. To compare with Shijiazhuang city, Figure 4 presents the time series of APIs for the four cities from 2010 to Jan. 14, 2013. In general, Shijiaz- huang city had the worst air quality that the average API 0% 10% 20% 30% 40% 50% 60% 70% 80% 90% 100% 2001 2002 2003 2004 2005 2006 2007 2008 2009 2010 2011 2012 % of the year Year >300 250-300 200 250 150-200 100-150 50 100 <=50 Figure 2. API distribution in Shijiazhuang city in 2001-2012. 0 50 100 150 200 250 300 350 1-1 1-7 1-13 1-19 1-25 1-31 2-6 2-12 2-18 2-24 3-1 3-7 3-13 3-19 3-25 3-31 4-6 4-12 4-18 4-24 4-30 5-6 5-12 5-18 5-24 5-30 6-5 6-11 6-17 6-23 6-29 7-5 7-11 7-17 7-23 7-29 8-4 8-10 8-16 8-22 8-28 9-3 9-9 9-15 9-21 9-27 10-3 10-9 10-15 10-21 10-27 11-2 11-8 11-14 11-20 11-26 12-2 12-8 12-14 12-20 12-26 API Date 2008 2009 2010 2011 2012 Figure 3. Time series of API in Shijiazhuang in 2008-2012. Copyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. 50 in Feb. 2012 to Jan. 2013 was 83.3. Then was Handan city, with the average API of 73.6 during the same period. Baoding and Tangshan city had the average numbers of 70.8 and 69.4, respectively. At the end of 2010, there was a severe pollution epi- sode in Shijiazhuang city, with the API of near 300 (as 420 μg·m−3 of daily average PM10). At the end of 2011, Shijiazhuang city didn’t show big difference in pollutant character from 2010, but a highly polluted episode hap- pened in Handan city that the largest API was as high as 348 (as 458 μg·m−3 of daily average PM10). In this month (Dec. 2011), the average APIs were 118.1, 102.9, 100.1 and 92.1 for Handan, Baoding, Tangshan and Shijiaz- huang, respectively. As discussed above, very severe haze pollution hap- pened over east China in the winter of 2012, in which Beijing-Tianjin-Hebei area was one of the most polluted regions. It is clearly indicated in Figure 4. The APIs reached the top limit, 500 (representing 600 μg·m−3 of daily average PM10). It is four times of the CNAAQS. One of the most possible reasons might be the special meteorological conditions, comparing with the former two years. Lots of investigations are needed before draw- ing a convictive conclusion of this episode. In Feb. 2012, the MEP released the new CNAAQS [7], which will be implemented in 2016, and the new techni- cal regulations on air quality daily reports [8]. In the new system, more pollutants, such as CO, O3 and PM2.5, are involved and API is replaced by Air Quality Index (AQI). From Jan. 2013, the MEP started to publish the real- time concentrations of SO2, NO2, CO, 1-hr and 8-hr O3, PM10 and PM2.5, as well as their AQIs, of all the national monitoring sites in the 74 cities including the capitals, major cities in Beijing-Tianjin-Hebei area, Yangtze River Delta, and Pearl River Delta (http://113.1 08.142.147: 20035/emcpublish/). At the same time the old daily APIs for those cities were stopped to update after Jan. 14, 2013. It is a progress that more detailed information on air quality can be accessed on the real time system, but it is a pity that up to now, the users could not access any longer history data except for the data for the past 24 hours. More understanding on the past special winter might be obtained when the historical real time data are accessible from the system. 2.2. Academic Observations The largest scale of air quality observations over the Bei- jing-Tianjin-Hebei area were pursued by the Institute of Atmospheric Physics, Chinese Academy of Science (IAP, CAS) [9]. 25 monitoring stations were established in northern China by IAP since 2009, out of which 16 were located in Hebei area [9], involving nine cities: Shijiaz- huang, Baoding, Tangshan, Hengshui, Cangzhou, Lang- fang, Chengde, Zhangjiakou, and Qinhuangdao. PM10, SO2 and NOX were observed in these stations. Table 1 summarizes the results of these studies and the observa- tions carried out by the other researchers. It is listed ac- cording to the locations of the observation sites, from the north to the south of Hebei. The northest site is Xinglong, located in the Chengde city. It is only the rural and background site in the table. The daily average concentrations of PM10, SO2, NOX and O3 didn’t exceed the present CNAAQS [6], neither the maximum daily concentrations. Only the maximum hour- ly O3 concentrations exceeded the standard (291 μg·m−3, 46% higher than the CNAAQS). O3 pollution at this background site is unnegligible according to the obser- vations [10], which may be induced by the large quanti- ties of pollutant emissions for the near huge cities. 0 100 200 300 400 500 API Date Tangshan Handan BaodingShijiazhuang Figure 4. Time series of API in Tangshan, Handan, Baoding and Shijiazhuang in 2010-2012. Copyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. 51 Table 1. Air quality observations in Hebei Province (unit: μg·m−3). Site Period Environment City size Region Daily PM10 Daily PM2.5 Daily SO2 Daily NO2 Daily NOX Daily O3 Hourly O3 Ref. Xinglong Aug. 15- Sep. 15 2006 Rural and background County-level city Chengde 69.4 (7.0 - 141.2)a- 4.4 (0.2 - 17.2) a- 15.1 (5.9 - 22.1)a - 137 (21 - 291)a[10] Xianghe Jun.-Sep. 2008 Rural County-level city Langfang 113 ± 52 (248)b 76 ± 42 (184)b 13.4 ± 15.2 (84.4)b 14.5 ± 8.6 (41.0)b 15.9 ± 9.1 (43.3)b 82 ± 38 (230)b - [11] Tangshan Jun.-Aug. 2007 Cultural and educational City Tangshan - 109.8 ± 26.4 - 41.7 ± 7.6 - 66.7 ± 16.8 157.8 ± 42.5 [12] Tangshan Sep.-Oct, 2007 Cultural and educational City Tangshan - 150.9 ± 58.1 - 46.0 ± 8.9 - 46.4 ± 25.8 123.5 ± 61.4 [12] Tangshan Jun.-Aug. 2008 Cultural and educational City Tangshan - 103.9 ± 50.3 44.8 ± 31.1 38.6 ± 10.5 - 74.6 ± 25.8 153.0 ± 52.8 [12] Tangshan Sep.-Oct. 2008 Cultural and educational City Tangshan - 91.9 ± 62.4 52.2 ± 25.2 40.4 ± 12.6 - 42.4 ± 21.4 108.3 ± 52.5 [12] Zhuozhou Jul. 2009- Feb. 2011 Cultural and educational County-level city Baoding 153 - 27 - 68 44 - [13] Baoding Jul. 2009- Feb. 2011 Cultural and educational City Baoding 189 - 72 - 83 48 - [13] Shijiazhuang Aug. 12- Sep. 25 2007 Cultural and educational Capital city Shijiazhuang- 114.5 ± 45.3 - 51.9 ± 11.0 - 81.3 ± 35.6 166.7 ± 67.1 [14] Shijiazhuang Jun.-Sep. 2008 Cultural and educational Capital city Shijiazhuang150.7 ± 62.1 99.4 ± 48.6 80.2 ± 36.6 43.9 ± 19.8 - 64.0 ± 33.9 148.6 ± 71.5 [14] Shijiazhuang Jul. 2009- Feb. 2011 Cultural and educational City Shijiazhuang204 - 87 - 74 34 - [13] Handan Aug.-Oct. 2012 Cultural and educational City Handan 196.5 ± 107.1 96.7 ± 55.2 69.2 ± 31.4 37.0 ± 26.3 66.3 ± 31.4 67.5 ± 22.9 135.8 ± 53.4 [15] Handan Nov.- Dec. 2012 Cultural and educational City Handan 248.6 ± 102.4 121.5 ± 60.4 142.4± 56.4 51.9 ± 12.5 130.0 ± 53.9 14. ± 8.6 40.5 ± 16.7 [15] Handan Jan. 2013 Cultural and educational City Handan 347.2 ± 174.6 233.4 ± 144.4 222.6± 86.5 93.3 ± 25.2 215.6 ± 72.7 8.8 ± 5.2 22.0 ± 14.8 [15] aThe data is “average(minimum-maximum)”; bThe data is “average ± standard deviation (maximum)”. Other data is “average” or “average ± standard devia- tion”. Xianghe site is in Langfang city, between Beijing and Tianjin city. The average PM10, SO2 and NOX didn’t ex- ceed the present daily standard during the summer of 2008, but the PM2.5 concentration were slightly higher than the new CNAAQS for daily PM2.5 concentrations (75 μg· m−3). Note that this was the Beijing Olympic pe- riod, during which air quality were much better than the normal situation. Tangshan is one of the heavy industry bases in China. From the Table 1 we can found that PM was the key pollutant in Tangshan. Even in the Olympic period (Jun.- Aug. 2008), the average PM2.5 concentration were 39% higher than the new standard for daily PM2.5. Zhuozhou and Baoding site showed the same characteristics that PM was the most important pollutant. Their average PM10 concentrations during Jul. 2009 to Feb. 2011 were 153 and 189 μg·m−3, respectively, much higher than the annual limit of PM10 (100 μg·m−3). SO2 in Baoding site exceeded the national annual standard (60 μg·m−3), and NOX in both Zhuozhou and Baoding site exceeded the new national annual standard (50 μg·m−3). According to Table 1, Shijiazhuang, the capital city of Hebei, and Handan, the southest city in Hebei, were the two most polluted cities. The PM10 and PM2.5 concentra- tions in all observed periods were exceeding the CNAAQS. In Shijiazhuang, the average PM10 concentra- tions were 204 μg·m−3 for Jul. 2009 to Feb. 2011, which was about two times of the present annual limit. PM2.5 concentration, even in Olympic period, was 1.3 times of new CNAAQS. Observation studies in Handan were pursued since Aug., 2012. The average PM10 and PM2.5 concentrations could reach 248.6 and 121.5 μg·m−3 in the Copyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. 52 winter of 2012, which is about 1.6 times of the present PM10 limit and the new standard for PM2.5. As discussed above, Jan. 2013 was quite special and highly polluted. During this month, the average PM10 and PM2.5 concen- trations were 347.2 and 233.4 μg·m−3, respectively, which were 2.3 and 3.1 times of the daily limit. SO2 and NOX in wintertime were also unnegligible in Shijiaz- huang and Handan city. SO2 pollution in Shijiazhuang was more severe than in Baoding, and NOX was on the contrary. Comparing with Handan, O3 pollution in Shiji- azhuang city was more serious according to the limited data. Long-term observations are needed to understand the air pollution characteristics in the southern Hebei cities. In intercomparison with other cities outside Hebei, Wu’s study [13] compared the PM10, SO2, NOX and O3 concentrations in Beijing, Zhuozhou (a county-level city within Baoding), Baoding and Shijiazhuang and con- cluded that during the monitoring period (Jul. 2009-Feb. 2011), Shijiazhuang city had highest concentrations of PM10 and SO2. The highest NOx concentrations appeared in Beijing and the most severe O3 pollution happened in Baoding. And during the three years, NOX concentrations were increasing and SO2’s were decreasing. O3 and PM10 concentrations kept stable. In [9], two severe pollution episodes over North China were reported in the period of Oct. 27 to Nov. 10 in 2009. In the comparison of Beijing, Tianjin and nine cities in Hebei (except Xingtai and Handan city), the highest daily PM10 concentration appeared in Shijiazhuang of 600 μg·m−3, four times of the national limit of 150 μg·m−3. Another important conclusion is that the heavy pollution episodes were characterized by nearly uniform concen- trations over northern China and directly related to the strength and duration of the southern flows. And the me- teorological conditions of light wind, temperature rever- sion and low mixed layer were important contributors to the increase of PM. In Liu et al.’s study [16], PM10 were sampled during Sep. to Oct. 2005 all over Hebei Province, Beijing and Tianjin City, to analysis the PAH pollution. They found that the highest PM10 concentration appeared in Handan and Shijiazhuang and the PAH pollution were most seri- ous in Handan, Shijiazhuang and Tangshan. In general, air pollution in the southern cities is more severe than in the northern cities in Hebei. PM is un- doubtedly the key pollutant. SO2 and NOX are unnegligi- ble and O3 pollution in larger cities is also significant, indicating that the both the coal-burning emissions and the mobile sources should be considered in the air pollu- tion controls. 2.3. Visibility and Haze Frequencies Visibility might be seen, to some extent, as an indicator of air quality. It has a longer history data for analysis. Che et al. gathered the visibility data from 1981 to 2005 of 615 meteorological stations in mainland China and found that 71% of these stations observed a visible dete- rioration and this trend became more clear after 1990 [17]. The highest haze frequencies happen in three areas: North China, the Yangtze River Delta and the Pearl River Delta. And the rapid increase in haze frequencies occurs in the middle and southern areas of North China Plain, the middle and lower reaches of the Yangtze River, and South China. The North China area has both the highest number of haze days and the most rapid growth in haze frequency [18]. Within North China area, Zhao [19] analyzed the data from 100 stations in Beijing-Tianjin-Hebei area from 1980 to 2008 and found that the southern cities in Hebei, such as Shijiazhuang, Xingtai and Handan had the lowest visibility of 10 - 14 km on annual average (Beijing was 15 - 20 km) since 1990. In comparison with other cities using the data from 743 stations all over China, the haze frequency in Xingtai City ranked second on average from 1951 to 2005, and became the first after the mid 1990s [20]. Wang et al. [18] analyzed the haze frequencies in 2001 to 2010 of the seven typical cities in North China, Bei- jing, Tianjin, Shijiazhuang, Xingtai, Taiyuan, Zhengzhou and Jinan. It was found that 2007 was the worst year and the haze frequencies from highest to lowest were Tai- yuan, Shijiazhuang, Zhengzhou, Xingtai, Jinan, Beijing, and Tianjin. 3. Air Pollution Control History and Emissions Hebei Province made a great effort on air pollution con- trol since 1998 [21]. In 1998, air pollution control meas- urements focused on the key corporations, key industries and key regions, such as tourist regions and areas along the high way. In 1999, eleven cities were all required to make the comprehensive air pollution control action plan, and the mobile emission controls were strengthened as well. In 2002, besides the continuous emission controls in major industries, the energy using in cities was paid more attention to and the central heating was pushed to spread in urban areas. In 2003, the provincial total amount con- trol of SO2 was started, according to the national control plan. But it was found that the pollution emissions didn’t decrease in the following three years, partially because of the unexpected rapid increase in energy consumption [22,23]. In 2007, Hebei government released the Action Plan of the Comprehensive Controls of Flue Gas Emissions in Hebei Province. It required all the emission instruments reached the national emission standards before Jun. 2008. Copyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. 53 The explosive increase in vehicle population in Hebei Province was noticed and its pollution control was streng- thened as well. In 2008, the objectives of the Action Plan were ac- complished and urban air quality was improved due to the flue gas cleaning, fugitive dust control and mobile source control. During the 2008 Beijing Olympics, lots of small industries, high-pollution plants were phase out or shutdown to ensure the good air quality in Beijing. It brought a better air quality in Hebei Province as well in this year. In 2009, the SO2 total amount control, energy optimizing in cities, moving high-pollution plants from our urban area were continuous pushing forward in He- bei Province. In 2010, the national SO2 emission control objective was successfully accomplished [23]. Regional air quality jointly control and prevention were brought forward by MEP. Hebei government published the regional air pol- lution control guideline to accelerate the regional scale air quality improvement. In the national 12th FYP of jointly air pollution pre- vention and control published in 2012, Beijing-Tianjin- Hebei was listed in the three key regions. More effective controls could be expected under this action structure. Figure 5 gives the provincial emissions of SO2, fly ash and dust emissions from 1998 to 2010. The data is come from the Report on the Environmental State of Hebei Province published every year by Hebei Environmental Protection Bureau (HBEPB) [21]. It can be seen that the total SO2 emissions decreased in 1998 to 2002 by 9.0% from the 1405 kt·y−1 to 1279 kt·y−1. Then it began to in- crease to 1545.5 kt·y−1 in 2006, which could partially attribute to the rapid increase of energy use during these five years [22,24]. After that it kept decreasing again, due to the effective national-scale SO2 emission controls during the 11th FYP (2006-2010) [23]. In 2010 the total SO2 emission was 1233.8 kt·y−1, which is 20.2% lower than that in 2006. Figure 5 also indicated that industry 1998 1999 20002001 2002 2003 2004 200520062007 2008 20092010 Yea SO2, domestic SO2, industry 0 200 400 600 800 1000 1200 1400 1600 1800 Fly ash, domestic Fly ash, industry Annual Emission (103 t y-1) dust, industry Figure 5. SO2, fly ash, and dust emissions in Hebei Province in 1998-2010. contributed most of the SO2 emissions in Hebei, which the fractions were between 80.6% (2010) to 86.7% (2007). The domestic emissions were relatively stable that kept between 186.4 kt·y−1 (2008) to 239.6 kt·y−1 (2010). As to fly ash emissions, the general trend was de- creasing, from 934 kt·y−1 in 1998 to 499.7 kt·y−1 in 2010. During 2001 to 2006 it kept relatively stable between 699 kt·y−1 to 738 kt·y−1. After that the decreasing trend was obvious from 723.2 kt·y−1 in 2006 by 30.9% to 499.7 kt·y−1 in 2010. The industrial emission also accounted for a big fraction of 63.6% (2009) to 80.0% (1998). The industrial dust emissions showed the similar variation as the SO2 emissions. The general trend was decreasing, from 1007 kt·y−1 in 1998 by 68.1% to 320.9 kt·y−1 in 2010. The rapid decrease happened during the 11th FYP (2006-2010) as well. 4. Conclusions Air pollution in Hebei Province has aroused a wide pub- lic concern, partially because of the severe fog-haze pe- riod happening in the beginning of 2013. It was reported that during this period, seven out of the top ten polluted cities in China were within Hebei Province. But, most of the previous studies involving Hebei focused on Bei- jing’s air quality, the impact of Hebei’s emissions to the air quality in Beijing, etc. Very few studies were pursued focusing on the severe air pollution within Hebei. In this study, we reviewed and analyzed the air pollu- tion history and status in Hebei Province, according to the API data and relative academic observations. It is concluded that air pollution in southern cities are much more severe than in northern cities. PM is the most im- portant pollutant in Hebei cities, and SO2 and NOX pollu- tion are unnegligible as well. O3 pollution in larger cities is significant, indicating that Hebei’s cities are on the way from the coal-burning pollution to the mixed-source pollution. Visibility and haze frequencies in Hebei cities are discussed, that Hebei has both the highest number of haze days and the most rapid growth in haze frequency in recent years. Hebei made a great effort on the air pollution control since 1998. The major air pollutant, such as SO2 and fly ash, showed a trend of increase in 2001 to 2006 and de- crease since 2006. In 2012 MEP published national plan of the regional jointly air pollution prevention and con- trol, more effective control strategies and measurement could be expected to improve the air quality in Hebei Province. 5. Acknowledgements This study was sponsored by the National Natural Sci- ence Foundation of China (No. 41105105) and the Natu- Copyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. 54 ral Science Foundation of Hebei Province (No. D2011 402019). REFERENCES [1] MEP, “China National Ambient Air Quality Standards,” GB3095-2012, MEP, Beijing, 2012. [2] NBS (Natural Bureau of Statistics), “China Statistical Yearbook 2012,” China Statistical Press, Beijing, 2012. [3] NBS (Natural Bureau of Statistics), “China Energy Statis- tical Yearbook 2012,” China Statistical Press, Beijing, 2012. [4] Q. Zhang, D. G. Streets, G. R. Carmichael, K. B. He, H. Huo, A. Kannari, Z. Klimont, I. S. Park, S. Reddy, J. S. Fu, D. Chen, L. Duan, Y. Lei, L. T. Wang and Z. L. Yao. “Asian Emissions in 2006 for the NASA INTEX-B Mis- sion,” Atmospheric Chemistry and Physics, Vol. 9, 2009, pp. 5131-5153. doi:10.5194/acp-9-5131-2009 [5] L. T. Wang, P. Zhang, S. B. Tan, X. J. Zhao, D. D. Cheng, W. Wei, J. Su and X. M. Pan, “Assessment of Urban Air Quality in China Using Air Pollution Indices (APIs),” Journal of the Air & Waste Management Association, Vol. 63, No. 2, 2013, pp. 170-178. doi:10.1080/10962247.2012.739583 [6] State Environmental Protection Agency of China, “China National Ambient Air Quality Standard (in Chinese),” GB3095-1996, State Environmental Protection Agency of China, Beijing, 1996. [7] State Environmental Protection Agency of China, “China National Ambient Air Quality Standard (in Chinese),” GB3095-2012, State Environmental Protection Agency of China, Beijing, 2012. [8] State Environmental Protection Agency of China, “Tech- nical Regulations on Ambient Air Quality Index (in Chi- nese),” HJ633-2012, State Environmental Protection Agency of China, Beijing, 2012. [9] D. S. Ji, Y. S. Wang, L. L. Wang, L. F. Chen, B. Hu, G. Q. Tang, J. Y. Xin, T. Song , T. X. Wen, Y. Sun, Y. P. Pan and Z. R. Liu, “Analysis of Heavy Pollution Episodes in Selected Cities of Northern China,” Atmospheric En- vironment, Vol. 50, 2012, pp. 338-348. doi:10.1016/j.atmosenv.2011.11.053 [10] T. X. Wen, Y. S. Wang, H. H. Xu, Z. Q. Ma and S. D. Ji. “Comparison of the Characteristics of Ambient Pollutant s in Urban and Background Region in Beijing during August and September (in Chinese),” Research of Envi- ronmental Sciences, Vol. 20, No. 5, 2007, pp. 7-11. [11] Y. P. Pan, Y. S. Wang, B. Hu, Q. Liu, Y. H. Wang and W. D. Nan, “Observation on Atmospheric Pollution in Xianghe During Beijing 2008 Olympic Games (in Chi- nese),” Environmental Science, Vol. 31, No. 1, 2010, pp. 1-9. [12] X. Y. Wang, J. Y. Xin, Y. S. Wang, X. X. Feng and Y. P. Zhang, “Observation and Analysis of Air Pollution in Tangshan During Summer and Autumn Time,” Environ- mental Science, Vol. 31, No. 4, 2010, pp. 877-885. [13] Y. Wu, “The Network Observation and Research on the Atmospheric Pollutants in Beijing, Zhuozhou, Baoding and Shijiazhuang,” Master’s Thesis, Nanjing University of Information Science &Technology, 2011. [14] W. P. Du, Y. S. Wang, T. Song, J. Y. Xin, Y. S. Cheng and D. S. Ji, “Characteristics of Atmospheric Pollutants during the Period of Summer and Autumn in Shijiaz- huang,” Environmental Science, Vol. 31, No. 7, 2010, pp. 1-8. [15] P. Zhang, S. B. Tan, L. T. Wang, X. J. Zhao, J. Su, F. F. Zhang, Z. Wei, W. Wei and D. D. Cheng. “Characteris- tics of Atmospheric Particulate Matter Pollution in Han- dan City,” Acta Scientiae Circumstantiae, (in Press). [16] S. Z. Liu, X. Q. Li, S. Tao, Z. F. Tian, J. F. Wang and Y. Gao, “PAHs in the Atmosphere from the Area of Hebei, Beijing, and Tianjin during the Non-Heating Season,” Acta Scientiae Circumstantiae, Vol. 28, No. 10, 2008, pp. 2105-2110. (in Chinese) [17] H. Z. Che, X. Y. Zhang, Y. Li, Z. J. Zhou, J. J. Qu and X. J. Hao, “Haze Trends over the Capital Cities of 31 Prov- inces in China, 1981-2005,” Theoretical and Applied Climatology, Vol. 97, No. 3-4, 2009, pp. 235-242. doi:10.1007/s00704-008-0059-8 [18] L. T. Wang, J. Xu, J. Yang, X. J. Zhao, W. Wei, D. D. Cheng, X. M. Pan and J. Su, “Understanding Haze Pollu- tion over the Southern Hebei Area of China Using the CMAQ Model,” Atmospheric Environment, Vol. 56, 2012, pp. 69-79. doi:10.1016/j.atmosenv.2012.04.013 [19] P. S. Zhao, X. L Zhang, X. F. Xu and X. J. Zhao, “Long-Term Visibility Trends and Characteristics in the Region of Beijing, Tianjin, and Hebei, China,” Atmos- pheric Research, Vol. 101, No. 3, 2011, pp. 711-718,. doi:10.1016/j.atmosres.2011.04.019 [20] D. Wu, X. J. Wu, F. Li, H. B. Tan, J. Chen, Z. Q. Cao, X. Sun, H. H. Chen, H. Y. Chen, “Temporal and spatial variation of haze during 1951-2005 in Chinese mainland (in Chinese),” Meteorologica Sinica, Vol. 68, 2010, pp. 680-688. [21] HBEPB, “Report on the Environmental State in Hebei Province, 1998-2010,” 2013. http://www.hb12369.net:8000/hjzlzkgb/ [22] L. T. Wang, C. Jang, Y. Zhang, K. Wang, Q. Zhang, D. Streets, J. Fu, Y. Lei, J. Schreifels, K. B. He, J. M. Hao, Y. F. Lam, J. Lin, N. Meskhidze, S. Voorhees, D. Evarts and S. Phillips, “Assessment of air Quality Benefits from National Air Pollution Control Policies in China. Part I: Background, Emission Scenarios and Evaluation of Me- teorological Predictions,” Atmospheric Environment, Vol. 44, No. 28, 2010, pp. 3442-3448. doi:10.1016/j.atmosenv.2010.05.051 [23] W. B. Xue, J. N. Wang, H. Niu, J. T. Yang, B. P. Han, Y. Lei, H. L. Chen and C. L. Jiang, “Assessment of Air Quality Improvement Effect under the National Total Emission Control Program during the Twelfth National Five-Year Plan in China,” Atmospheric Environment, Vol. 68, No., 2013, pp. 74-81. doi:10.1016/j.atmosenv.2012.11.053 [24] L. T. Wang, C. Jang, Y. Zhang, K. Wang, Q. Zhang, D. Streets, J. Fu, Y. Lei, J. Schreifels, K. B. He, J. M. Hao, Y. F. Lam, J. Lin, N. Meskhidze, S. Voorhees, D. Evarts and S. Phillips, “Assessment of Air Quality Benefits from Copyright © 2013 SciRes. OJAP
L.-T. WANG ET AL. Copyright © 2013 SciRes. OJAP 55 National Air Pollution Control Policies in China. Part II: Evaluation of Air Quality Predictions and Air Quality Be- nefits Assessment,” Atmospheric Environment, Vol. 44, No. 28, 2010, pp. 3449-3457. doi:10.1016/j.atmosenv.2010.05.058
|